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The Development of Catalysis

E-BookPDF2 - DRM Adobe / Adobe Ebook ReaderE-Book
352 Seiten
Englisch
John Wiley & Sonserschienen am27.02.20171. Auflage
This book gradually brings the reader, through illustrations of the most crucial discoveries, into the modern world of chemical catalysis. Readers and experts will better understand the enormous influence that catalysis has given to the development of modern societies.
•    Highlights the field's onset up to its modern days, covering the life and achievements of luminaries of the catalytic era
•    Appeals to general audience in interpretation and analysis, but preserves the precision and clarity of a scientific approach
•    Fills the gap in publications that cover the history of specific catalytic processes


Adriano Zecchina, Ph.D, is Professor Emeritus of the University of Turin, where he was full professor of physical chemistry from 1975 to 2009. He is a member of the National Academy of Lincei and Academia Europaea. His research is mainly devoted to studying the surface properties of catalytic materials with spectroscopic methods.
Salvatore Califano, Ph.D, is the director of the European Laboratory of Molecular Spectroscopy in Florence, Italy. His main research focuses on dynamics of molecular crystals and determination of the lifetime of phonons and vibrons by pico- and femtosecond spectroscopy or by high-resolution infrared and Raman spectroscopy.mehr
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E-BookPDF2 - DRM Adobe / Adobe Ebook ReaderE-Book
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Produkt

KlappentextThis book gradually brings the reader, through illustrations of the most crucial discoveries, into the modern world of chemical catalysis. Readers and experts will better understand the enormous influence that catalysis has given to the development of modern societies.
•    Highlights the field's onset up to its modern days, covering the life and achievements of luminaries of the catalytic era
•    Appeals to general audience in interpretation and analysis, but preserves the precision and clarity of a scientific approach
•    Fills the gap in publications that cover the history of specific catalytic processes


Adriano Zecchina, Ph.D, is Professor Emeritus of the University of Turin, where he was full professor of physical chemistry from 1975 to 2009. He is a member of the National Academy of Lincei and Academia Europaea. His research is mainly devoted to studying the surface properties of catalytic materials with spectroscopic methods.
Salvatore Califano, Ph.D, is the director of the European Laboratory of Molecular Spectroscopy in Florence, Italy. His main research focuses on dynamics of molecular crystals and determination of the lifetime of phonons and vibrons by pico- and femtosecond spectroscopy or by high-resolution infrared and Raman spectroscopy.
Details
Weitere ISBN/GTIN9781119181309
ProduktartE-Book
EinbandartE-Book
FormatPDF
FormatFormat mit automatischem Seitenumbruch (reflowable)
Erscheinungsjahr2017
Erscheinungsdatum27.02.2017
Auflage1. Auflage
Seiten352 Seiten
SpracheEnglisch
Dateigrösse10400 Kbytes
Artikel-Nr.3018257
Rubriken
Genre9201

Inhalt/Kritik

Inhaltsverzeichnis
1;Cover;1
2;Title Page;5
3;Copyright;6
4;Contents;7
5;Preface;11
6;Chapter 1 From the Onset to the First Large-Scale Industrial Processes;13
6.1;1.1 Origin of the Catalytic Era;13
6.2;1.2 Berzelius and the Affinity Theory of Catalysis;16
6.3;1.3 Discovery of the Occurrence of Catalytic Processes in Living Systems in the Nineteenth Century;18
6.4;1.4 Kinetic Interpretation of Catalytic Processes in Solutions: The Birth of Homogeneous Catalysis;20
6.5;1.5 Onset of Heterogeneous Catalysis;30
6.6;1.6 First Large-Scale Industrial Processes Based on Heterogeneous Catalysts;38
6.6.1;1.6.1 Sulfuric Acid Synthesis;38
6.6.2;1.6.2 Ammonia Problem;41
6.6.3;1.6.3 Ammonia Oxidation Process;44
6.6.4;1.6.4 Ammonia Synthesis;45
6.7;1.7 Fischer-Tropsch Catalytic Process;52
6.8;1.8 Methanol Synthesis;56
6.9;1.9 Acetylene Production and Utilization;58
6.10;1.10 Anthraquinone Process for Hydrogen Peroxide Production;59
6.11;References;61
7;Chapter 2 Historical Development of Theories of Catalysis;71
7.1;2.1 Heterogeneous Catalysis;71
7.2;2.2 Chemical Kinetics and the Mechanisms of Catalysis;74
7.3;2.3 Electronic Theory of Catalysis: Active Sites;84
7.4;References;88
8;Chapter 3 Catalytic Processes Associated with Hydrocarbons and the Petroleum Industry;95
8.1;3.1 Petroleum and Polymer Eras;95
8.2;3.2 Catalytic Cracking, Isomerization, and Alkylation of Petroleum Fractions;96
8.3;3.3 Reforming Catalysts;103
8.4;3.4 Hydrodesulfurization (HDS) Processes;105
8.5;3.5 Hydrocarbon Hydrogenation Reactions with Heterogeneous Catalysts;106
8.6;3.6 Olefin Polymerization: Ziegler-Natta, Metallocenes, and Phillips Catalysts;110
8.7;3.7 Selective Oxidation Reactions;121
8.7.1;3.7.1 Alkane Oxidation;121
8.7.2;3.7.2 Olefin Oxidation;122
8.7.3;3.7.3 Aromatic Compounds Oxidation;123
8.8;3.8 Ammoximation and Oxychlorination of Olefins;125
8.9;3.9 Ethylbenzene and Styrene Catalytic Synthesis;129
8.10;3.10 Heterogeneous Metathesis;130
8.11;3.11 Catalytic Synthesis of Carbon Nanotubes and Graphene from Hydrocarbon Feedstocks;131
8.12;References;133
9;Chapter 4 Surface Science Methods in the Second Half of the Twentieth Century;143
9.1;4.1 Real Dispersed Catalysts versus Single Crystals: A Decreasing Gap;143
9.2;4.2 Physical Methods for the Study of Dispersed Systems and Real Catalysts;144
9.3;4.3 Surface Science of Single-Crystal Faces and of Well-defined Systems;151
9.4;References;159
10;Chapter 5 Development of Homogeneous Catalysis and Organocatalysis;167
10.1;5.1 Introductory Remarks;167
10.2;5.2 Homogeneous Acid and Bases as Catalysts: G. Olah Contribution;168
10.3;5.3 Organometallic Catalysts;173
10.4;5.4 Asymmetric Epoxidation Catalysts;187
10.5;5.5 Olefin Oligomerization Catalysts;191
10.6;5.6 Organometallic Metathesis;192
10.7;5.7 Cross-Coupling Reactions;198
10.8;5.8 Pd(II)-Based Complexes and Oxidation of Methane to Methanol;202
10.9;5.9 Non-transition Metal Catalysis, Organocatalysis, and Organo-Organometallic Catalysis Combination;203
10.9.1;5.9.1 Metal-Free Hydrogen Activation and Hydrogenation;204
10.9.2;5.9.2 Amino Catalysis;205
10.10;5.10 Bio-inspired Homogeneous Catalysts;206
10.11;References;207
11;Chapter 6 Material Science and Catalysis Design;217
11.1;6.1 Metallic Catalysts;217
11.2;6.2 Oxides and Mixed Oxides;220
11.2.1;6.2.1 SiO2 and SiO2-Based Catalysts and Processes;221
11.2.2;6.2.2 Al2O3 and Al2O3-Based Catalysts and Processes;223
11.2.3;6.2.3 SiO2-Al2O3- and SiO2-Al2O3-Based Catalysts and Processes;223
11.2.4;6.2.4 MgO- and MgO-Based Catalysts and Processes;224
11.2.5;6.2.5 ZrO2 and ZrO2-Based Catalysts and Processes;224
11.3;6.3 Design of Catalysts with Shape and Transition-State Selectivity;225
11.4;6.4 Zeolites and Zeolitic Materials: Historical Details;226
11.5;6.5 Zeolites and Zeolitic Materials Structure;230
11.6;6.6 Shape-Selective Reactions Catalyzed by Zeolites and Zeolitic Materials;233
11.6.1;6.6.1 Alkanes- and Alkene-Cracking and Isomerization;234
11.6.2;6.6.2 Aromatic Ring Positional Isomerizations;235
11.6.3;6.6.3 Synthesis of Ethyl Benzene, Cumene, and Alkylation of Aromatic Molecules;236
11.6.4;6.6.4 Friedel-Crafts Acylation of Aromatic Molecules;237
11.6.5;6.6.5 Toluene Alkylation with Methanol;237
11.6.6;6.6.6 Asaki Process for Cyclohexanol Synthesis;238
11.6.7;6.6.7 Methanol-to-Olefins (MTO) Process;238
11.6.8;6.6.8 Nitto Process;239
11.6.9;6.6.9 Butylamine Synthesis;239
11.6.10;6.6.10 Beckman Rearrangements on Silicalite Catalyst;239
11.6.11;6.6.11 Partial Oxidation Reactions Using Titanium Silicalite;239
11.6.12;6.6.12 Nylon-6 Synthesis: The Role of Zeolitic Catalysts;241
11.6.13;6.6.13 Pharmaceutical Product Synthesis;241
11.7;6.7 Organic-Inorganic Hybrid Zeolitic Materials and Inorganic Microporous Solids;242
11.7.1;6.7.1 Organic-Inorganic Hybrid Zeolitic Materials;242
11.7.2;6.7.2 ETS-10: A Microporous Material Containing Monodimensional TiO2 Chains;243
11.7.3;6.7.3 Hydrotalcites: Microporous Solids with Exchangeable Anions;244
11.8;6.8 Microporous Polymers and Metal-Organic Frameworks (MOFs);244
11.8.1;6.8.1 Microporous Polymers;244
11.8.2;6.8.2 Metal-organic Frameworks;246
11.9;References;247
12;Chapter 7 Photocatalysis;255
12.1;7.1 Photochemistry and Photocatalysis: Interwoven Branches of Science;255
12.2;7.2 Photochemistry Onset;257
12.3;7.3 Physical Methods in Photochemistry;261
12.4;7.4 Heterogeneous and Homogeneous Photocatalysis;263
12.5;7.5 Natural Photosynthesis as Model of Photocatalysis;265
12.6;7.6 Water Splitting, CO2 Reduction, and Pollutant Degradation: The Most Investigated Artificial Photocatalytic Processes;268
12.6.1;7.6.1 Water Splitting;269
12.6.2;7.6.2 CO2 Photoreduction;273
12.6.3;7.6.3 Photocatalysis in Environmental Protection;275
12.7;References;276
13;Chapter 8 Enzymatic Catalysis;281
13.1;8.1 Early History of Enzymes;281
13.2;8.2 Proteins and Their Role in Enzymatic Catalysis;285
13.3;8.3 Enzymes/Coenzymes Structure and Catalytic Activity;296
13.4;8.4 Mechanism of Enzyme Catalysis;300
13.5;8.5 Biocatalysis;306
13.6;References;307
14;Chapter 9 Miscellanea;311
14.1;9.1 Heterogeneous and Homogeneous Catalysis in Prebiotic Chemistry;311
14.2;9.2 Opportunities for Catalysis in the Twenty-First Century and the Green Chemistry;324
14.3;References;329
15;Index;333
16;EULA;344mehr