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E-BookPDF1 - PDF WatermarkE-Book
Englisch
Springer International Publishingerschienen am24.01.20152015
This book presents the latest advances in ultrafast science, including both ultrafast optical technology and the study of ultrafast phenomena. It covers picosecond, femtosecond, and attosecond processes relevant to applications in physics, chemistry, biology, and engineering. Ultrafast technology has a profound impact in a wide range of applications, amongst them biomedical imaging, chemical dynamics, frequency standards, material processing, and ultrahigh-speed communications. This book summarizes the results presented at the 19th International Conference on Ultrafast Phenomena and provides an up-to-date view of this important and rapidly advancing field.mehr
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E-BookPDF1 - PDF WatermarkE-Book
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Produkt

KlappentextThis book presents the latest advances in ultrafast science, including both ultrafast optical technology and the study of ultrafast phenomena. It covers picosecond, femtosecond, and attosecond processes relevant to applications in physics, chemistry, biology, and engineering. Ultrafast technology has a profound impact in a wide range of applications, amongst them biomedical imaging, chemical dynamics, frequency standards, material processing, and ultrahigh-speed communications. This book summarizes the results presented at the 19th International Conference on Ultrafast Phenomena and provides an up-to-date view of this important and rapidly advancing field.

Inhalt/Kritik

Inhaltsverzeichnis
1;Preface;6
2;Contents;8
3;Contributors;32
4;Part I Attosecond and High-Order HarmonicGeneration and Applications;82
5;1 Attosecond Control of Electron Emission in Two-Color Ionization of Atoms;83
5.1;Abstract;83
5.2;1 Introduction;83
5.3;2 Results and Discussion;84
5.4;3 Conclusions;86
5.5;Acknowledgments;86
5.6;References;86
6;2 Probing Xenon Electronic Structure by Two-Color Driven High-Order Harmonic Generation;87
6.1;Abstract;87
6.2;1 Introduction;87
6.3;2 The Giant Resonance in Xenon;88
6.4;3 Experimental Results;88
6.5;4 Conclusions;90
6.6;References;90
7;3 Strong Field Applications of Gigawatt Self-compressed Pulses from a Kagome Fiber;91
7.1;Abstract;91
7.2;References;95
8;4 Intense Attosecond Pulses for Probing Ultrafast Molecular Dynamics;96
8.1;Abstract;96
8.2;1 Introduction;96
8.3;2 Nonlinear Fourier Transformation Spectroscopy with Intense Attosecond Pulse Train;97
8.4;3 Generation of Multi-gigawatt Isolated Attosecond Pulses;98
8.5;References;98
9;5 Disentangling Structural and Dynamical Effects via Multidimensional High Harmonic Spectroscopy;100
9.1;Abstract;100
9.2;1 Introduction;100
9.3;2 Experimental Setup and Results;101
9.4;References;103
10;6 Attosecond Frequency Resolved Momentum Imaging of Two-Photon Dissociative Ionization Dynamics of Nitrogen Molecule;104
10.1;Abstract;104
10.2;1 Introduction;104
10.3;2 Experimental Setup;105
10.4;3 Results and Discussion;105
10.5;Acknowledgments;107
10.6;References;107
11;7 High-Order Harmonics Fourier Transform Spectroscopy of Two-Photon Dissociative Ionization of Hydrogen Molecules;108
11.1;Abstract;108
11.2;1 Introduction;108
11.3;2 Experimental;109
11.4;3 Results and Discussion;110
11.5;Acknowledgments;111
11.6;References;111
12;8 Simultaneous Observation of Vibrational Wavepackets of Nitrogen Molecule in Neutral and Singly-Charged Manifolds;112
12.1;Abstract;112
12.2;1 Introduction;112
12.3;2 Experimental Setup;113
12.4;3 Results and Discussion;113
12.5;Acknowledgments;115
12.6;References;115
13;9 Photo Ionization Time Delay in Molecular Hydrogen;116
13.1;Abstract;116
13.2;1 Introduction;116
13.3;2 Setup;117
13.4;3 Results;117
13.5;References;119
14;10 Ultrafast Relaxation and Photodissociation Dynamics of 1,3-Butadiene Studied by Probing Molecular Orbitals;120
14.1;Abstract;120
14.2;References;123
15;11 Ultrafast and Photodissociation Dynamics of 1,2-Butadiene Studied by Photoelectron Spectroscopy;124
15.1;Abstract;124
15.2;References;127
16;12 Direct Comparison of Multi-photon and EUV Single-Photon Probing of Molecular Relaxation Processes;128
16.1;Abstract;128
16.2;1 Introduction;128
16.3;2 Experimental;129
16.4;3 Results and Discussion;129
16.5;Acknowledgments;130
16.6;References;131
17;13 Sub-4-fs Charge Migration in Phenylalanine;132
17.1;Abstract;132
17.2;Acknowledgments;134
17.3;References;135
18;14 Recombination-Induced Autoionization Process in Rare-Gas Clusters;136
18.1;Abstract;136
18.2;1 Introduction;136
18.3;2 Experiment;137
18.4;3 Results and Discussion;137
18.5;References;139
19;15 X-Ray Magnetic Circular Dichroism Probed Using High Harmonics;140
19.1;Abstract;140
19.2;References;143
20;16 Extreme Ultraviolet Transient Grating Measurement of Insulator-Metal Transition Dynamics in VO2;144
20.1;Abstract;144
20.2;1 Introduction;144
20.3;2 Experiment;145
20.4;3 Results;145
20.5;Acknowledgments;147
20.6;References;147
21;17 Delayed Core-Level Photoemission from the van der Waals Crystal WSe2;148
21.1;Abstract;148
21.2;1 Introduction;148
21.3;2 Experimental Setup;149
21.4;3 Results and Discussion;149
21.5;References;151
22;18 Optimization of Quantum Trajectories Driven by Strong-Field Waveforms;152
22.1;Abstract;152
22.2;References;157
23;19 Phase-Matched Generation of High Order Harmonic for Study of Molecular Dynamics;158
23.1;Abstract;158
23.2;1 Introduction;158
23.3;2 Experimental Results and Discussions;159
23.4;References;161
24;20 Multiphoton Transitions for Robust Delay-Zero Calibration in Attosecond Transient Absorption;163
24.1;1 Introduction;163
24.2;2 Results;164
24.3;3 Conclusion and Outlook;164
24.4;References;166
25;21 Infrared Double Optical Gating for Generating Submicrojoule Isolated Attosecond Pulses;167
25.1;Abstract;167
25.2;1 Introduction;167
25.3;2 High-Energy Continuum Harmonic Spectra;168
25.4;References;170
26;22 Generation of Isolated Soft X-Ray Pulses Around the Carbon K-Edge Using CEP-Stabilized Few-Cycle IR Pulses;171
26.1;Abstract;171
26.2;1 Introduction;171
26.3;2 CEP-Dependent HHG;172
26.4;3 Pressure Dependence of HH Spectra;173
26.5;4 Conclusion;174
26.6;References;174
27;23 Bright Isolated Attosecond Soft X-Ray Pulses;175
27.1;Abstract;175
27.2;Acknowledgement;178
27.3;References;178
28;24 Strong-Field-Enhanced Forward Scattering of High-Order Harmonics;179
28.1;Abstract;179
28.2;References;182
29;Part II Atomic, Molecular and OpticalSciences-Gas Phase;183
30;25 Non-adiabatic Effects in Electron Momenta;184
30.1;Abstract;184
30.2;1 Strong Field Ionization;184
30.3;2 Field Intensity Calibration;185
30.4;3 Quantitative Comparison of Theory and Experiment;185
30.5;4 Conclusion and Outlook;186
30.6;Acknowledgements;186
30.7;References;187
31;26 Determination of Absolute Cross-Sections of Nonresonant EUV-UV Two-Color Two-Photon Ionization of He;188
31.1;Abstract;188
31.2;1 Introduction;188
31.3;2 Experimental;189
31.4;3 Results and Discussion;190
31.5;References;191
32;27 Attosecond Spatial Control of Electron Wave Packet Emission Dynamics;192
32.1;Abstract;192
32.2;1 Introduction;192
32.3;Acknowledgements;195
32.4;References;196
33;28 Probing Elastic Rescattering Through Half-Cycle Cutoffs in Above-Threshold Ionization Spectra;197
33.1;Abstract;197
33.2;1 Introduction;197
33.3;2 Experimental Setup;198
33.4;3 Analysis and Conclusions;198
33.5;References;200
34;29 Experimental Signature of Light Induced Conical Intersections in Diatomics;201
34.1;Abstract;201
34.2;Acknowledgments;203
34.3;References;203
35;30 Sub-femtosecond Steering of Carbon Hydrogen Bonds;205
35.1;Abstract;205
35.2;1 Introduction;205
35.3;2 CEP Dependent Asymmetry of the Deprotonation in Acetylene Dication;206
35.4;3 Mechanism of the Directional Control via the CEP;207
35.5;References;208
36;31 Tabletop Imaging of Structural Evolutions in Chemical Reactions;209
36.1;Abstract;209
36.2;1 Introduction;209
36.3;2 Results and Discussion;210
36.4;References;212
37;32 Structure Dependence of Kinetic Energy Released in X-ray-Induced Fragmentation;213
37.1;Abstract;213
37.2;Acknowledgments;215
37.3;References;216
38;33 Controlling Fragmentation Reactions of Polyatomic Molecules with Impulsive Laser Alignment;217
38.1;Abstract;217
38.2;Acknowledgments;221
38.3;References;221
39;34 Intense Field Ionization of C2H2 and 12C13CH2 Aligned in Field-Free Space;222
39.1;Abstract;222
39.2;1 Introduction;222
39.3;2 Experiment;223
39.4;3 Results and Discussion;223
39.5;References;225
40;35 Ionization of Aligned O2 by Intense Laser Pulse;226
40.1;Abstract;226
40.2;1 Introduction;226
40.3;2 Experiment;227
40.4;3 Results and Discussion;227
40.5;References;228
41;36 Strong-Field Electronic Control of Multiple-Bond Breaking Dynamics in Ethylene;229
41.1;Abstract;229
41.2;Acknowledgments;233
41.3;References;233
42;37 Electronic Pre-determination of Ethylene Fragmentation Dynamics;234
42.1;Abstract;234
42.2;Acknowledgments;237
42.3;References;238
43;38 Long-Lived Neutral H _{2} in Hydrogen Migration Within Hydrocarbon Dication;239
43.1;Abstract;239
43.2;1 Introduction;239
43.3;2 Results and Discussion;240
43.4;References;242
44;39 Pump-Probe Photoelectron Imaging with 90-nm Excitation Pulses;243
44.1;Abstract;243
44.2;1 Introduction;243
44.3;2 Experiments and Results;244
44.4;3 Conclusions;246
44.5;References;246
45;40 Time-Resolved Coulomb Explosion Imaging of Ultrafast Fragmentation of CS2 in Highly Charged States;247
45.1;Abstract;247
45.2;1 Introduction;247
45.3;2 Experiment;248
45.4;3 Results and Discussion;249
45.5;4 Conclusion;249
45.6;References;249
46;41 Initial Phase Shifts in the Quantum Beat Resulting from the Ultrafast Internal Conversion of Pyrazine;251
46.1;Abstract;251
46.2;1 Introduction;251
46.3;2 Results;252
46.4;3 Conclusions;253
46.5;References;254
47;42 Ab Initio Quantum Dynamical Study on Ultrafast Nonradiative Transition Pathways of Pyrazine;255
47.1;Abstract;255
47.2;1 Introduction;255
47.3;2 Computational Outline;256
47.4;3 Results and Discussion;257
47.5;References;258
48;43 The Ultrafast Wolff Rearrangement in the Gas Phase;259
48.1;Abstract;259
48.2;1 Introduction;259
48.3;2 Experimental Results;259
48.4;3 Conclusion;261
48.5;References;261
49;44 Time-Resolved Photoelectron Spectroscopy and Ab Initio Multiple Spawning Studies of Hexamethylcyclopentadiene;263
49.1;Abstract;263
49.2;1 Introduction;263
49.3;2 Methods;264
49.4;3 Results and Discussion;264
49.5;References;266
50;45 Laser-Assisted Electron Diffraction for Probing Femtosecond Nuclear Dynamics of Gas-Phase Molecules;267
50.1;Abstract;267
50.2;1 Introduction;267
50.3;2 Experiment;268
50.4;3 Results and Discussion;268
50.5;4 Conclusion;269
50.6;References;270
51;46 Filament-Driven Lasing Action for Combustion Diagnosis;271
51.1;Abstract;271
51.2;1 Introduction;271
51.3;2 Experimental Results and Discussion;272
51.4;3 Summary;273
51.5;References;273
52;Part III Solid State Physics and Chemistry;275
53;47 Anomalous Phase Change in [(GeTe)2/(Sb2Te3)]20 Superlattice Observed by Coherent Phonon Spectroscopy;276
53.1;Abstract;276
53.2;1 Introduction;276
53.3;2 Experiment;277
53.4;3 Result;277
53.5;4 Discussion;278
53.6;5 Conclusion;278
53.7;References;278
54;48 Dynamical Coupling of Rabi Oscillation to Coherent Phonon in Semiconductor Microcavities;279
54.1;Abstract;279
54.2;1 Introduction;279
54.3;2 Experiment;280
54.4;3 Experimental Results and Discussion;280
54.5;References;282
55;49 Coherent Control Over Two-Dimensional Lattice Vibrational Trajectories in alpha -Quartz Using Polarization Pulse Shaping;283
55.1;Abstract;283
55.2;1 Introduction;283
55.3;2 Methods;284
55.4;3 Results;285
55.5;4 Discussion and Conclusion;285
55.6;References;286
56;50 Ultrafast Lattice Dynamics of Phase-Change Materials Monitored by a Pump-Pump-Probe Technique;287
56.1;Abstract;287
56.2;1 Introduction;287
56.3;2 Experimental;288
56.4;3 Results and Discussion;288
56.5;4 Summary;289
56.6;Acknowledgement;289
56.7;References;290
57;51 Enhancement of Superconducting Coherence in YBa2Cu3Ox by Resonant Lattice Excitation;291
57.1;Abstract;291
57.2;References;294
58;52 Coherent Phonon Dynamics in Singlet Fission of Rubrene Single Crystal;295
58.1;Abstract;295
58.2;1 Introduction;295
58.3;2 Experimental Methods;296
58.4;3 Results and Discussion;296
58.5;Acknowledgments;297
58.6;References;298
59;53 Acceleration of Ultrafast Singlet Fission in Aza-Derivative of TIPS-Pentacene;299
59.1;Abstract;299
59.2;1 Introduction;299
59.3;2 Experimental Details;300
59.4;3 Results and Discussion;300
59.5;References;302
60;54 Vibrational Coherence Reveals the Role of Dark Multiexciton States in Ultrafast Singlet Exciton Fission;303
60.1;Abstract;303
60.2;References;306
61;55 Ultrafast Carriers Dynamics in Silicon: A Joint Experimental and Theoretical Study;307
61.1;Abstract;307
61.2;Acknowledgments;309
61.3;References;309
62;56 Ultrabroadband Infrared Pump-Probe Spectroscopy Using Chirped-Pulse Upconversion;310
62.1;Abstract;310
62.2;References;312
63;57 Investigation of Laser-Induced Currents in Large-Band-Gap Dielectrics;314
63.1;Abstract;314
63.2;1 Introduction;314
63.3;2 Experimental Setup and Results;315
63.4;3 Conclusion and Outlook;316
63.5;References;317
64;58 Field-Induced Dynamics of Correlated Electrons in LiH and NaBH4;318
64.1;Abstract;318
64.2;1 Introduction;318
64.3;2 Results;319
64.4;References;320
65;59 Spontaneous Formation of Correlated Charge Coherence Induced by 1.5-Cycle Pulse in 1-D Organic Metal (TMTTF)2AsF6;321
65.1;Abstract;321
65.2;1 Introduction;321
65.3;2 Experiment;322
65.4;3 Results and Discussions;322
65.5;4 Summary;324
65.6;References;324
66;60 Coherent Dynamics of Structural Symmetry During the Ultrafast Melting of a Charge Density Wave;325
66.1;Abstract;325
66.2;1 Introduction;325
66.3;2 Experimental;326
66.4;3 Results and Discussion;326
66.5;References;327
67;61 10 fs Dynamics of Photoinduced Magnetic Transition in Double-Layered Charge Ordering in LuFe2O4 Under Interlayer Excitation;329
67.1;Abstract;329
67.2;1 Introduction;329
67.3;2 Experiment;330
67.4;3 Results and Discussions;330
67.5;4 Summary;332
67.6;References;333
68;62 Magnetically Induced Lattice Dynamics in a Magnetoelectric Antiferromagnet Cr2O3;334
68.1;Abstract;334
68.2;1 Introduction;334
68.3;2 Sample and Experiment;334
68.4;3 Result and Discussion;335
68.5;References;336
69;63 Coherent Magnetism: Pushing the Limits of Spin-Photon Interaction;337
69.1;Abstract;337
69.2;1 Introduction;337
69.3;2 9 fs Magneto Optical Four Wave Mixing Experiment;338
69.4;3 Microscopic Origin of the Magneto-optical Coherent Emission;339
69.5;Acknowledgement;340
69.6;References;340
70;64 Quantum Droplets of Electrons and Holes in GaAs Quantum Wells;341
70.1;Abstract;341
70.2;References;343
71;65 Exciton Dynamics in Cu-Doped InAs Colloidal Quantum Dots;344
71.1;Abstract;344
71.2;1 Introduction;344
71.3;2 Experiments;345
71.4;3 Conclusions;346
71.5;References;347
72;66 Rabi Oscillations in an InAs Quantum Dot Ensemble Observed in Pre-pulse 2D Coherent Spectroscopy;348
72.1;Abstract;348
72.2;1 Introduction;348
72.3;2 Results and Discussion;349
72.4;References;351
73;67 Slow Electron Cooling Dynamics of Highly Luminescent CdSxSe1-x Alloy Quantum Dot;352
73.1;Abstract;352
73.2;1 Introduction;352
73.3;2 Results and Discussion;353
73.4;3 Conclusion;354
73.5;References;355
74;68 Ultrafast Dynamics Related to Spin Crossover Processes in Single Crystal [FeII(bpy)3](PF6)2;356
74.1;Abstract;356
74.2;1 Introduction;356
74.3;2 Experimental Methods;357
74.4;3 Results and Discussion;358
74.5;References;359
75;69 Femtosecond Electron Diffraction Study of the Spin Crossover Dynamics of Single Crystal [Fe(PM-AzA)2](NCS)2;360
75.1;Abstract;360
75.2;1 Introduction;360
75.3;2 Experimental Methods;362
75.4;3 Results and Discussion;362
75.5;Acknowledgements;362
75.6;References;363
76;70 Ab Initio Solution of Structural Dynamics with Ultrafast Electron Diffraction and Charge Flipping;364
76.1;Abstract;364
76.2;1 Introduction;364
76.3;2 Experimental Methods;365
76.4;3 Preliminary Results;366
76.5;References;367
77;71 Laser Streaking of Free-Electron Pulses at 25 keV;368
77.1;Abstract;368
77.2;1 Introduction;368
77.3;2 Concept, Experiment, Results;369
77.4;3 Conclusions;371
77.5;References;371
78;72 Ultrafast Single-Electron Diffraction;372
78.1;Abstract;372
78.2;1 Introduction;372
78.3;2 Single-Electron Pulse Compression;373
78.4;3 Time-Resolved Single-Electron Diffraction;374
78.5;4 Conclusions;375
78.6;References;375
79;Part IV Interfacial, Surface, Thin Filmsand Carbon Nanotubes;376
80;73 Hydrated Phospholipid Surfaces Probed by Ultrafast 2D Spectroscopy of Phosphate Vibrations;377
80.1;Abstract;377
80.2;References;379
81;74 Femtosecond Time and Angle Resolved Photoemission Spectroscopy of Liquids;381
81.1;Abstract;381
81.2;Acknowledgments;383
81.3;References;384
82;75 Ultrafast Vibrational Dynamics of Water at a Zwitterionic Lipid/Water Interface Revealed by Two-Dimensional Heterodyne-Detected Vibrational Sum Frequency Generation (2D HD-VSFG);385
82.1;Abstract;385
82.2;1 Introduction;385
82.3;2 Experimental Methods;386
82.4;3 Results and Discussion;387
82.5;References;388
83;76 Ultrafast Vibrational Spectroscopy at Liquid Interfaces by Heterodyne-Detected Sum-Frequency Generation;389
83.1;Abstract;389
83.2;1 Introduction;389
83.3;2 Infrared-Excited TR-HD-VSFG and 2D HD-VSFG to Study Ultrafast Vibrational Dynamics at Liquid Interfaces;390
83.4;3 Ultraviolet-Excited TR-HD-VSFG to Study Ultrafast Photochemical Dynamics at Liquid Interfaces;391
83.5;References;392
84;77 Ultrafast Electron Solvation at the Room Temperature Ionic Liquid/Metal Interface;393
84.1;Abstract;393
84.2;1 Introduction;393
84.3;2 Results and Discussion;394
84.4;3 Conclusions;396
84.5;References;396
85;78 Ultrafast Spectroscopy Reveals Bulk Heterojunction Morphology;397
85.1;Abstract;397
85.2;1 Introduction;397
85.3;2 Experimental;398
85.4;3 Results;398
85.5;References;400
86;79 Toward Ultrafast In Situ X-ray Studies of Interfacial Photoelectrochemistry;401
86.1;Abstract;401
86.2;1 Introduction;401
86.3;2 Experiments and Results;402
86.4;Acknowledgment;404
86.5;References;404
87;80 Ultrafast Dynamics in Epitaxial Silicene on Ag(111);405
87.1;Abstract;405
87.2;Acknowledgments;407
87.3;References;407
88;81 Accessing Energy-Dependent Photoemission Delays in Solids;409
88.1;Abstract;409
88.2;1 Introduction;409
88.3;2 Results;410
88.4;3 Conclusion and Outlook;411
88.5;References;412
89;82 Visualization of Ultrafast Electron Dynamics Using Time-Resolved Photoemission Electron Microscopy;413
89.1;Abstract;413
89.2;1 Introduction;413
89.3;2 Experimental;414
89.4;3 Results;414
89.4.1;3.1 Carrier Lifetime in a Si Nanowire;415
89.4.2;3.2 Electron Drift Velocity and Mobility on a GaAs Surface [3];415
89.5;References;416
90;83 A New Regime of Nanoscale Thermal Transport: Collective Diffusion Counteracts Dissipation Inefficiency;417
90.1;Abstract;417
90.2;1 Introduction;417
90.3;2 A New Regime of Nanoscale Thermal Transport;418
90.4;3 The Experiment;419
90.5;4 Characterizing Phonon Transport in Materials;419
90.6;Acknowledgments;420
90.7;References;420
91;84 Laser-Induced Plasma Dynamics Imaged by Femtosecond In-Line Holography;421
91.1;Abstract;421
91.2;1 Experimental Setup and Numerical Approach;421
91.3;2 Results and Discussion;422
91.4;Acknowledgments;423
91.5;References;423
92;85 Resonant Optical Kerr Response with Ultrashort Decay Time by Nonlocal Wave Coupling of Light and Excitons;424
92.1;Abstract;424
92.2;1 Experimental Procedures;425
92.3;2 Results and Discussion;425
92.4;Acknowledgments;427
92.5;References;427
93;86 Single-Shot Real-Time Observation of Ultrafast Amorphization in Ge2Sb2Te5 Thin Film;428
93.1;Abstract;428
93.2;1 Introduction;428
93.3;2 Experimental Method;429
93.4;3 Results and Discussion;430
93.5;4 Summary;430
93.6;Acknowledgments;430
93.7;References;431
94;87 Electrochemical Control of Coherent Phonon Generations in Single-Walled Metallic Carbon Nanotubes;432
94.1;Abstract;432
94.2;1 Introduction;432
94.3;2 Experiments;433
94.4;3 Results and Discussion;433
94.5;4 Conclusion;434
94.6;References;435
95;88 Ultrafast Charge Photogeneration and Dynamics in Semiconducting Carbon Nanotubes;436
95.1;Abstract;436
95.2;Acknowledgments;438
95.3;References;438
96;89 Thickness Dependent Hot-phonon Effects Observed by Femtosecond Mid-infrared Luminescence in Graphene;439
96.1;Abstract;439
96.2;1 Introduction;439
96.3;2 Experiment;440
96.4;3 Results and Discussion;440
96.5;References;442
97;Part V Chemistry-Liquid Phase;443
98;90 Discriminating Racemic from Achiral Solutions with Femtosecond Accumulative Spectroscopy;444
98.1;Abstract;444
98.2;1 Introduction;444
98.3;2 Measurement Principle and Experimental Results;444
98.4;3 Discussion and Outlook;446
98.5;References;447
99;91 Quantum Dynamics of Molecular Reactions Directed by Explicit Solvent Environment;448
99.1;Abstract;448
99.2;1 Ultrafast Chemical Reactions in Solution;448
99.3;2 Photochemical Bond Cleavage in Acetonitrile;449
99.4;3 Solvent Potential Extracted from Classical Molecular Dynamics Simulations;449
99.5;4 Quantum Dynamics in the Combined Potential of the Molecule and Its Surrounding;451
99.6;References;452
100;92 Excited-State Dynamics of Catalytically Active Transition Metal Complexes Studied by Transient Photofragmentation in Gas Phase and Transient Absorption in Solution;453
100.1;Abstract;453
100.2;1 Introduction;453
100.3;2 Results and Discussion;454
100.4;3 Conclusions;455
100.5;Acknowledgments;456
100.6;References;456
101;93 Coherent Control of the Photodissociation of Triiodide in Solution Reveals New Pathways;457
101.1;Abstract;457
101.2;1 Introduction;457
101.3;2 Experimental Methods;458
101.4;3 Results and Discussion;458
101.5;Acknowledgments;460
101.6;References;460
102;94 Multidimensional Photochemistry Model: Application to Aminobenzonitrile and Benzopyran;461
102.1;Abstract;461
102.2;1 Aminobenzonitrile (ABN, R = H) versus Dimethylaminobenzonitrile (DMABN, R = CH3) Charge Transfer;462
102.3;2 Photoisomerisation of Benzopyran (the Spiropyran Chromophore);464
102.4;References;465
103;95 Tuning of Isomerization Rates in Indigo-Based Photoswitches;466
103.1;Abstract;466
103.2;1 Introduction;466
103.3;2 Experimental;467
103.4;3 Results and Discussions;467
103.5;References;469
104;96 Bimolecular Reactions on a Timescale Below 1 ps;470
104.1;Abstract;470
104.2;1 Beating Diffusion to Get Access to the Intrinsic Rates of Bimolecular Reactions;470
104.3;2 Tuning Reactivity to Speed up Reaction Times;471
104.4;References;473
105;97 Ultrafast Dynamics of a Bistable Intramolecular Proton Transfer Switch;474
105.1;Abstract;474
105.2;1 Introduction;474
105.3;2 Results;475
105.4;3 Discussion;475
105.5;References;477
106;98 Excited State Structural Dynamics Probed with Time-Resolved Sulfur K-Edge X-Ray Absorption Spectroscopy;478
106.1;Abstract;478
106.2;1 Introduction;478
106.3;2 Transient Sulfur K-Edge Spectroscopy;479
106.4;3 Summary;481
106.5;References;481
107;99 Solvent Environment Revealed by Positively Chirped Pulses;482
107.1;Abstract;482
107.2;1 Introduction;482
107.3;2 Experimental;483
107.4;3 Results and Discussion;483
107.5;References;485
108;100 Coherent Wavepacket Motion in Ultrafast Intermolecular Electron Transfer in Electron-Donating Solvent;486
108.1;Abstract;486
108.2;1 Introduction;486
108.3;2 Results and Discussion;487
108.4;3 Conclusion;489
109;101 Elementary Electron and Ion Dynamics in Ionized Liquid Water;490
109.1;Abstract;490
109.2;1 Introduction;490
109.3;2 Experimental Methods;491
109.4;3 Results and Discussion;491
109.5;Acknowledgments;492
109.6;References;493
110;102 Signatures of Conical Intersection Mediated Relaxation Dynamics in Time-Resolved Broadband Raman Detection;494
110.1;Abstract;494
110.2;1 Ultrafast Relaxation Dynamics of RNA and DNA Bases;494
110.3;2 Off-Resonant Raman Detection Schemes;495
110.4;3 Time-Resolved Raman Signatures of Conical Intersection Mediated Relaxation of Uracil;495
110.5;Acknowledgments;497
110.6;References;498
111;103 VIPER 2D-IR: Novel Pulse Sequence to Track Exchange Beyond the Vibrational Lifetime;499
111.1;Abstract;499
111.2;1 Mixed IR/Vis 2D Spectroscopies;499
111.3;2 Viper 2D-IR;500
111.4;References;502
112;104 Sagnac Interferometer for Two-Dimensional Spectroscopy in the Pump-Probe Geometry;503
112.1;Abstract;503
112.2;Acknowledgments;506
112.3;References;506
113;105 Broadband Electronic Two-Dimensional Spectroscopy in the Deep UV;507
113.1;Abstract;507
113.2;1 Introduction;507
113.3;2 Experimental Setup;508
113.4;3 Results and Discussion;509
113.5;References;510
114;106 A Non time Ordered Pulse Scanning Protocol for Multidimensional Spectroscopy with Entangled Light;511
114.1;Abstract;511
114.2;1 Introduction: Spectroscopy with Entangled Light;511
114.3;2 LOP---A New Non time Ordered Delay Scanning Protocol;512
114.4;3 Probing Intraband Dephasing Rates of Excitons in Aggregates;513
114.5;Acknowledgements;514
114.6;References;514
115;107 Ultrafast Interaction of Dark and Bright Electronic States in Open-Chain Carotenoids Investigated by Pump-DFWM;515
115.1;Abstract;515
115.2;1 Introduction;515
115.3;2 Experimental;516
115.4;3 Results and Discussion;516
115.5;References;518
116;108 Following the Excited State Dynamics of beta -Apo-82032-Carotenal with Two-Dimensional Electronic-Vibrational Spectroscopy;519
116.1;Abstract;519
116.2;1 Introduction;519
116.3;2 Experimental;520
116.4;3 Results and Discussion;521
116.5;4 Conclusions;521
116.6;Acknowledgments;522
116.7;References;522
117;109 Survival of Nuclear Coherences for a Series of Internal Conversions in Free Base Tetraphenylporphyrin;523
117.1;Abstract;523
117.2;1 Introduction;523
117.3;2 Results and Discussion;524
117.4;References;526
118;110 Distinctive Spectral Features of Exciton and Excimer States in the Ultrafast Electronic Deactivation of the Adenine Dinucleotide;527
118.1;Abstract;527
118.2;1 Introduction;527
118.3;2 Experimental Results;528
118.4;3 Discussion and Conclusions;529
118.5;Acknowledgments;529
118.6;References;529
119;111 Influence of Intramolecular Hydrogen Bonding on the Photodynamics of 2-(1-Ethynylpyrene)-Adenosine (PyA);530
119.1;Abstract;530
119.2;1 Introduction;530
119.3;2 Materials and Methods;531
119.4;3 Results;531
119.5;4 Discussion;532
119.6;References;532
120;112 S2 to S1 Relaxation Dynamics in Perylene Bisimide Dye Aggregates and Monomers;534
120.1;Abstract;534
120.2;1 Introduction;534
120.3;2 Experimental Approach;535
120.4;3 Analysis of the Dynamics;535
120.5;References;536
121;113 2D IR Spectroscopy with Phase-Locked Pulse Pairs from a Birefringent Delay Line;537
121.1;Abstract;537
121.2;Acknowledgments;540
121.3;References;540
122;114 Hydrogen Bond Dynamics in Alcohols Studied by 2D IR Spectroscopy;541
122.1;Abstract;541
122.2;1 Introduction;541
122.3;2 Experiment;542
122.4;3 Theory;542
122.5;4 Results and Discussion;542
122.6;References;545
123;115 Hydrogen Bond Enhancement of Fermi Resonances Explored with Ultrafast IR Two-Colour Pump-Probe and 2D-IR Spectroscopy;546
123.1;Abstract;546
123.2;References;548
124;116 Observation of the Dark State in Ruthenium Complexes Using Femtosecond Infrared Vibrational Spectroscopy;550
124.1;Abstract;550
124.2;1 Introduction;550
124.3;2 Experimental;551
124.4;3 Results and Discussion;552
124.5;References;553
125;117 Vibrational Dynamics of Nitrosyl Stretch of Ru Complex in Aqueous Solution Studied by Two-Dimensional Infrared Spectroscopy;554
125.1;Abstract;554
125.2;1 Introduction;554
125.3;2 Results and Discussion;555
125.4;References;557
126;118 Ultrafast IR Spectroscopy of O-H Stretching Modes in 2-Naphthol-Acetonitrile Photoacid-Base Complexes;558
126.1;Abstract;558
126.2;References;561
127;119 Vibrational Dynamics of the CN Stretching in the Electronically Excited State by UV and Visible-Pump and Infrared-Probe Spectroscopy;562
127.1;Abstract;562
127.2;1 Introduction;562
127.3;2 Results and Discussion;563
127.4;3 Conclusion;565
127.5;Part IVInterfacial, Surface, Thin Filmsand Carbon Nanotubes;376
127.6;References;565
128;120 Structural Motifs of Liquid Acetic Acid from Ultrafast CARS Spectroscopy;567
128.1;Abstract;567
128.2;1 Introduction;567
128.3;2 CO Vibration of Acetic Acid;568
128.4;References;569
129;121 Ultrafast Time-Domain Raman Study to Visualize Large-Amplitude Distortions in Copper Complexes;570
129.1;Abstract;570
129.2;1 Introduction;570
129.3;2 Experimental;571
129.4;3 Results and Discussion;572
129.5;References;573
130;122 Investigation of Vibrational Dynamics by Femtosecond Time-Resolved CARS;574
130.1;Abstract;574
130.2;Acknowledgments;577
130.3;References;577
131;123 Two-Dimensional Fourier Transform Infrared-Visible and Infrared-Raman Spectroscopies;578
131.1;Abstract;578
131.2;Acknowledgments;580
131.3;References;580
132;Part VI Biological Systems;581
133;124 Ultrafast Intersystem Crossing in SO2 and Nucleobases;582
133.1;Abstract;582
133.2;1 Introduction;582
133.3;2 Methodology;583
133.4;3 Results;583
133.4.1;3.1 Dynamics of SO2;584
133.4.2;3.2 Dynamics of DNA Nucleobases;584
133.5;4 Conclusion;585
133.6;References;586
134;125 Detection of the G(--H)2022 Radical in the Electronic Deactivation of the G--C Watson-Crick Base Pair;587
134.1;Abstract;587
134.2;1 Introduction;587
134.3;2 Experimental Details;588
134.4;3 Results and Discussion;588
134.5;Acknowledgments;589
134.6;References;589
135;126 Ultrafast Photoisomerization of Chiral Biomimetic Molecular Switches;590
135.1;Abstract;590
135.2;1 Introduction;590
135.3;2 Results;591
135.4;3 Discussion;592
135.5;References;593
136;127 Snapshots of Sub-picosecond Dynamics in Heme-proteins Captured by Femtosecond Stimulated Raman Scattering;594
136.1;Abstract;594
136.2;1 Background and Significance;594
136.3;2 Methods;595
136.4;3 Results;596
136.5;References;596
137;128 Vibrational Dynamics in Photoactive Yellow Protein Revealed by Mid-IR Pump/Visible Probe Spectroscopy;597
137.1;Abstract;597
137.2;1 Introduction;597
137.3;2 Experimental;598
137.4;3 Results and Discussion;598
137.5;4 Conclusion;599
137.6;References;600
138;129 Probing Ultrafast Structural Dynamics of Photoactive Yellow Protein with Femtosecond Time-Domain Raman Spectroscopy;601
138.1;Abstract;601
138.2;1 Introduction;601
138.3;2 Experimental;602
138.4;3 Results and Discussion;602
138.5;References;604
139;130 Vibrational Energy Flow in Hemeproteins;605
139.1;Abstract;605
139.2;1 Introduction;605
139.3;2 Vibrational Energy Flow in Cytochrome c [4];606
139.4;3 Vibrational Energy Flow in Myoglobin;606
139.5;4 Advantages of the Present Technique for Studies on Intermolecular Vibrational Energy Transfer in Condensed Phases;607
139.6;Acknowledgements;607
139.7;References;607
140;131 Towards Direct Measurement of Ultrafast Vibrational Energy Flow in Proteins;608
140.1;Abstract;608
140.2;References;611
141;132 Time-Resolved Impulsive Raman Study of Excited State Structures of Green Fluorescent Protein;612
141.1;Abstract;612
141.2;1 Introduction;612
141.3;2 Experimental Method;613
141.4;3 Results and Discussion;613
141.5;References;615
142;133 Nonlinear Fourier-Transform Spectroscopy Using Ultrabroadband Femtosecond Pulses for the Measurement of Photobleaching of Fluorescent Proteins;616
142.1;Abstract;616
142.2;1 Introduction;616
142.3;2 Nonlinear Fourier-Transform Spectroscopy;617
142.4;3 Experimental;617
142.5;4 Conclusions;619
142.6;Acknowledgements;619
142.7;References;619
143;134 Femtosecond Vibrational Spectroscopic Study on Photoexcitation Dynamics of DNO-Bound Myoglobin;620
143.1;Abstract;620
143.2;1 Introduction;620
143.3;2 Experimental Methods;621
143.4;3 Results and Discussion;621
143.5;References;623
144;Part VII Charge and EnergyTransfer-Photovoltaicand Light Harvesting;624
145;135 Interpreting Oscillations in Numerically Exact Simulations of 2D Electronic Spectra;625
145.1;Abstract;625
145.2;1 Introduction;625
145.3;2 Model;626
145.4;3 Results and Discussion;627
145.5;4 Conclusions;627
145.6;Acknowledgments;628
145.7;References;628
146;136 Coherent Ultrafast Charge Transfer in an Organic Photovoltaic Blend;629
146.1;Abstract;629
146.2;1 Introduction;630
146.3;2 Results;630
146.4;3 Conclusions;632
146.5;References;632
147;137 Ultrafast Energy and Charge Transfer Processes in a Flexible Molecular Triad Designed for Organic Photovoltaics;633
147.1;Abstract;633
147.2;1 Introduction;633
147.3;2 Results;634
147.4;3 Conclusions;635
147.5;References;635
148;138 Ultrafast Electron and Hole Dynamics in Novel Conjugated Star-Shaped Molecules;636
148.1;Abstract;636
148.2;1 Introduction;636
148.3;2 Experimental and Results;637
148.4;References;639
149;139 Photoinduced Charge Transfer Occurs Naturally in DNA;640
149.1;Abstract;640
149.2;1 Introduction;640
149.3;2 Results and Discussion;641
149.4;3 Conclusion;643
149.5;References;643
150;140 A Regulation of Energy Flow in Purple Bacterial Photosynthetic Antennas;644
150.1;Abstract;644
150.2;1 Introduction;644
150.3;2 Experimental;645
150.4;3 Results and Discussion;646
150.5;References;647
151;141 Elucidation and Control of Ultrafast Intramolecular Charge Transfer Dynamics of Marine Photosynthetic Pigments;648
151.1;Abstract;648
151.2;1 Introduction;648
151.3;2 Experimental;649
151.4;3 Results and Discussion;650
151.5;References;651
152;142 The Primary Photosynthetic Energy Conversion in Bacterial Reaction Centers---Stepwise Electron Transfer and the Effect of Elevated Exposure Levels;652
152.1;Abstract;652
152.2;1 The Primary Reactions of Photosynthetic Reaction Centers;652
152.3;2 Techniques;653
152.4;3 Results;653
152.5;References;654
153;143 Resonant Stimulated X-Ray Raman Spectroscopy of Molecule Following Core Ionization;656
153.1;Abstract;656
153.2;1 Introduction;656
153.3;2 Results and Discussion;657
153.4;Acknowledgments;658
153.5;References;658
154;144 Light Harvesting Dynamics in Gloeobacter Rhodopsin (GR);659
154.1;Abstract;659
154.2;1 Introduction;659
154.3;2 Experimental Methods;660
154.4;3 Results and Discussion;660
154.5;4 Conclusion;661
154.6;References;662
155;145 Disentangling Electronic and Vibrational Coherence in the Phycocyanin-645 Light-Harvesting Complex;663
155.1;Abstract;663
155.2;1 Introduction;663
155.3;2 Results and Discussion;664
155.4;3 Conclusions;665
155.5;References;665
156;146 Ultrafast Energy Flow and Equilibration Dynamics in Photosynthetic Light-Harvesting Complexes;667
156.1;Abstract;667
156.2;References;670
157;147 Primary Process in Light-Harvesting Complex Studied by Pump-Repump-Probe Spectroscopy;671
157.1;Abstract;671
157.2;1 Introduction;671
157.3;2 Experimental;672
157.4;3 Results and Discussion;672
157.5;4 Conclusion;674
157.6;References;674
158;148 Ultrabroadband Two-Dimensional Spectroscopy by a Birefringent Delay Line;675
158.1;Abstract;675
158.2;Acknowledgments;677
158.3;References;678
159;Part VIII THz Generation and Application;679
160;149 Filling the Entire Terahertz Frequency Gap by Single-Cycle MV/Cm Pulses;680
160.1;Abstract;680
160.2;1 Introduction;680
160.3;2 Experimental Results;680
160.4;References;682
161;150 Terahertz Imaging with Optical Resolution by Femtosecond Laser Filament in Air;683
161.1;Abstract;683
161.2;1 Introduction;683
161.3;2 Experimental Results;683
161.3.1;2.1 THz Sub-wavelength Imaging by Femtosecond Laser Filament;683
161.3.2;2.2 Resolution of THz Imaging (Diameter of THz Beam Emission from Femtosecond Laser Filament);685
161.4;3 Numerical Simulation;685
161.5;References;686
162;151 Ultrafast Optical Modulation of Efficiently-Generated Terahertz-Wave in Charge Ordered Organic Ferroelectrics;687
162.1;Abstract;687
162.2;1 Introduction;687
162.3;2 Experiments;688
162.4;3 Results and Discussions;688
162.5;References;690
163;152 Ultrafast Terahertz Response of Lithium Niobate in the Nonperturbative Regime;691
163.1;Abstract;691
163.2;1 Introduction;691
163.3;2 Experiment and Results;692
163.4;3 Discussion;693
163.5;References;693
164;153 Inherent Resistivity of Graphene to Strong THz Fields;694
164.1;Abstract;694
164.2;1 Introduction;694
164.3;2 Measurement;695
164.4;3 Results and Discussion;695
164.5;4 Conclusion;696
164.6;References;696
165;154 Nonlinear Carrier Responses in Gold Thin Films Induced by Intense Terahertz Waves;697
165.1;Abstract;697
165.2;1 Introduction;697
165.3;2 Experiments;698
165.4;3 Results and Discussion;698
165.5;4 Conclusions;700
165.6;References;700
166;155 THz-Controlled Photoelectron Emission from Nanotips;701
166.1;Abstract;701
166.2;1 Introduction;701
166.3;2 Experimental Methods;702
166.4;3 Results and Discussion;702
166.5;References;703
167;156 Nonlinear Carrier Dynamics in Semi-metal Bismuth Induced by Intense Terahertz Field;704
167.1;Abstract;704
167.2;1 Introduction;704
167.3;2 Experiment;705
167.4;3 Result and Discussion;706
167.5;4 Conclusion;706
167.6;References;707
168;157 Ultrafast Insulator-Metal Transition in VO2 Driven by Intense Multi-THz Pulses;708
168.1;Abstract;708
168.2;References;711
169;158 Coherent Ultrafast Magnetization Dynamics Non-resonantly Induced in Cobalt by an Intense Terahertz Transient;712
169.1;Abstract;712
169.2;1 Introduction;712
169.3;2 Experimental Results;713
169.4;References;715
170;159 Beating of Terahertz Pulse Induced Spin Precession in ErFeO3;716
170.1;Abstract;716
170.2;1 Introduction;716
170.3;2 Result;717
170.4;3 Conclusion;719
170.5;References;719
171;160 Resonant Antiferromagnetic Spin Wave Excitation by Terahertz Magnetic Near-Field with Split Ring Resonator;720
171.1;Abstract;720
171.2;1 Introduction;720
171.3;2 Experimental Setup;721
171.4;3 Results;722
171.5;4 Summary;723
171.6;References;723
172;161 Ultrafast Spin Dynamics in an Antiferromagnet NiO Observed in Pump-Probe and Terahertz Experiments;724
172.1;Abstract;724
172.2;1 Introduction;724
172.3;2 Sample;725
172.4;3 Experiment;725
172.5;4 Result and Discussion;725
172.6;References;726
173;Part IX Photoemitted Electron, Plasmonand Nanoplasmas;728
174;162 Controlling the Motion of Strong-Field, Few-Cycle Photoemitted Electrons in the Near-Field of a Sharp Metal Tip;729
174.1;Abstract;729
174.2;1 Introduction;729
174.3;2 Experimental Setup;730
174.4;3 Results;731
174.5;4 Conclusion;731
174.6;References;732
175;163 Velocity Map Imaging of Electrons Strong-Field Photoemitted from Si-Nanotip Arrays;733
175.1;Abstract;733
175.2;Acknowledgments;736
175.3;References;736
176;164 Visualization of Photocurrents in Nanoobjects by Ultrafast Low-Energy Electron Point-Projection Imaging;737
176.1;Abstract;737
176.2;1 Introduction;737
176.3;2 Method;738
176.4;3 Results and Discussion;739
176.5;4 Conclusions;740
176.6;References;740
177;165 Visualization of Charge Carrier Motion in Semiconductor Nanowires with Ultrafast Pump-Probe Microscopy;741
177.1;Abstract;741
177.2;1 Introduction;741
177.3;2 Pump-Probe Microscopy;741
177.4;Acknowledgments;743
177.5;References;744
178;166 Ultrafast Optical Control of Charge Dynamics in Organic and Hybrid Electronic Nanodevices;745
178.1;Abstract;745
178.2;References;748
179;167 Ultrafast Non-thermal Response of Plasmonic Resonance in Gold Nanoantennas;749
179.1;Abstract;749
179.2;References;752
180;168 Control of Femtosecond Surface Plasmon Coupled onto a Gold Tapered Tip and Its Nonlinear Emission;753
180.1;Abstract;753
180.2;1 Introduction;753
180.3;2 Experimental Setup;754
180.4;3 Results and Discussion;755
180.5;References;756
181;169 Ultrafast Optical-Field Controlled Photoemission from Plasmonic Nanoparticle Arrays;757
181.1;Abstract;757
181.2;References;759
182;170 Real Space and Real Time Observation of Plasmon Wavepacket Dynamics in Single Gold Nanorod;761
182.1;Abstract;761
182.2;1 Introduction;761
182.3;2 Experiment;762
182.4;3 Results and Discussion;762
182.5;References;763
183;171 Vector Pulse Shaped Ultrafast Plasmon Based on Response Functions Measured for Orthogonally Polarized Excitation;764
183.1;Abstract;764
183.2;1 Introduction;764
183.3;2 Experimental Setup;765
183.4;3 Results and Discussion;765
183.5;References;767
184;172 Few-Cycle Laser Pulse Induced Plasmon Assisted Thermionic Injection in Metal-Insulator-Metal Junctions;768
184.1;Abstract;768
184.2;1 Introduction;768
184.3;2 Experimental Setup;769
184.4;3 Results and Discussion;769
184.5;References;771
185;173 Single Nanoparticles and Nanoplasmas in Femtosecond Laser Fields;772
185.1;Abstract;772
185.2;1 Introduction and Summary;772
185.3;2 Experiment;773
185.4;3 Shock Waves in Nanoplasmas;773
185.5;4 Mapping Nanoscale Light Absorption with Plasma Explosion Imaging;775
185.6;5 Conclusion;776
185.7;References;776
186;Part X Novel Pulsed Sourcesand Application;777
187;174 Passively CEP-Stable Front End for Frequency Synthesis;778
187.1;References;781
188;175 Tunable Few-Cycle Mid-IR Pulses Towards Single-Cycle Duration by Adiabatic Frequency Conversion;782
188.1;Abstract;782
188.2;References;785
189;176 Carrier-Envelope Phase of Single-Cycle Pulses Generated Through Two-Color Laser Filamentation;786
189.1;Abstract;786
189.2;References;788
190;177 Phase-Locked Multi-THz High-Harmonic Generation by Dynamical Bloch Oscillations in Bulk Semiconductors;790
190.1;Abstract;790
190.2;References;793
191;178 Direct Generation of 7 fs Whitelight Pulses from Bulk Sapphire;794
191.1;Abstract;794
191.2;1 New Insights into Bulk Filamentation;794
191.3;2 Propagation Properties of New Frequencies and Generation of Sub-10-fs Pulses During SCG;795
191.4;3 Conclusion and Outlook;797
191.5;References;797
192;179 Ultrafast 2 00B5m Laser Oscillators Based on Thulium-Doped ZBLAN Fibers;798
192.1;Abstract;798
192.2;References;800
193;180 Characterizing Phase Fluctuations of Fiber Oscillators by Using External Optical Cavities;801
193.1;Abstract;801
193.2;1 Introduction;801
193.3;2 Experimental Setup and Results;802
193.4;3 Conclusion;803
193.5;References;804
194;181 Two Novel Schemes for Photon-Number Squeezed Pulse Generation in Ultrafast Nonlinear Fiber Optics;805
194.1;Abstract;805
194.2;1 Introduction;805
194.3;2 Photon Number Squeezing by Noise Reduced 1.5 mu m EDFA with the CBD Technique;806
194.4;3 Photon Number Squeezing by 800 nm Pulses with Spectral Narrowing;807
194.5;4 Conclusion;807
194.6;References;808
195;182 Towards a Compact Fiber Laser for Multimodal Imaging;809
195.1;Abstract;809
195.2;1 Introduction;809
195.3;2 Experimental;810
195.4;3 Results and Discussion;810
195.5;References;812
196;183 Measurement and Characterization of Sub-5 fs Broadband UV Pulses in the 230--350 nm Range;813
196.1;Abstract;813
196.2;1 Introduction;813
196.3;2 Experimental Layout;814
196.4;3 Results and Discussion;815
196.5;References;816
197;184 Generation and Characterization of Tunable 00B5J-Level, Sub-10 fs UV Pulses;818
197.1;Abstract;818
197.2;References;821
198;185 Femtosecond Pulses in 375--405 nm Region by Chirped Sum Frequency;822
198.1;Abstract;822
198.2;1 Introduction;822
198.3;2 Experimental;823
198.4;3 Results and Discussion;823
198.5;4 Conclusions;825
198.6;References;825
199;186 Pushing the NOPA to New Frontiers: Output to Below 400 nm, MHz Operation and ps Pump Duration;826
199.1;Abstract;826
199.2;1 Optical Parametric Amplifiers Pumped by Yb-Based Lasers;826
199.3;2 Fully Utilizing the Tuning Possibility of a 343 nm Pumped NOPA;827
199.4;3 Continuum-Seeded NOPA with 1 ps 130 W Pump Pulses;828
199.5;4 Towards New Applications of Wavelength-Tunable MHz 10 fs Pulses;829
199.6;References;829
200;187 2 MHz Tunable Non Collinear Optical Parametric Amplifiers with Pulse Durations Down to 6 fs;830
200.1;Abstract;830
200.2;1 Introduction;830
200.3;2 Results;831
200.4;3 Conclusions;833
200.5;References;833
201;188 Fiber-Slab-Pumped OPCPA for XUV-Based Time-Resolved Photoelectron Spectroscopy at 500 kHz Repetition Rate;835
201.1;Abstract;835
201.2;1 Introduction;835
201.3;2 Fiber Oscillator and Hybrid Fiber-Slab Amplifier;836
201.4;3 OPCPA Results and Discussion;837
201.5;References;838
202;189 Sub-100 fs Mid-Infrared Pulses as Driver for a Table-Top Hard X-Ray Source;839
202.1;Abstract;839
202.2;1 Introduction;839
202.3;2 Results;840
202.4;References;842
203;190 Generation of Stationary On-Axis Optical Filaments by Means of Dammann Lenses;843
203.1;Abstract;843
203.2;1 Introduction;843
203.3;2 Experimental Set-up;844
203.4;3 Experimental Results;845
203.5;4 Conclusions Results;846
203.6;References;846
204;191 Wavefront Analysis of High-Efficiency, Large-Scale, Thin Transmission Gratings;848
204.1;Abstract;848
204.2;1 Introduction;848
204.3;2 Design and Analysis of Transmission Gratings;849
204.4;3 Spatial Distortion and Wavefront Analysis;849
204.5;4 Ray Tracing and Summary;851
204.6;References;851
205;Part XI Pulse Shaping and Manipulations;852
206;192 High-Energy Sub-Optical-Cycle Parametric Waveform Synthesizer;853
206.1;Abstract;853
206.2;References;856
207;193 Above-Millijoule Optical Waveforms Compressible to Sub-fs Using Induced-Phase Modulation in a Neon-Filled Hollow-Core Fiber;857
207.1;Abstract;857
207.2;References;860
208;194 Isolating Quantum Coherence Using Coherent Multi-dimensional Spectroscopy with Spectrally Shaped Pulses;861
208.1;Abstract;861
208.2;1 Introduction;861
208.3;2 Experimental and Results;862
208.4;3 Conclusions;863
208.5;References;864
209;195 Spatiotemporal Dynamics of Femtosecond Pulses Shaped by Diffractive Optical Elements;865
209.1;Abstract;865
209.2;References;867
210;196 Spectral Shaping and Continuous Tuning of Multi-color Carrier-Envelope Phase Locked Pulse;869
210.1;Abstract;869
210.2;1 Introduction;869
210.3;2 Experimental;870
210.4;3 Results and Discussion;870
210.5;4 Summary;871
210.6;Acknowledgments;872
210.7;References;872
211;197 Tailoring of High-Field Multi-THz Waveforms with Sub-cycle Precision;873
211.1;Abstract;873
211.2;References;875
212;198 Over 1-mJ Intense Ultrashort Optical-Vortex Pulse Generation with Programmable Topological-Charge Control by Chirped-Pulse Amplification;877
212.1;Abstract;877
212.2;1 Introduction;877
212.3;2 Experiments and Results;878
212.4;References;880
213;199 The Influence of Generalized Focusing on Polarization-Shaped Few-Cycle Pulsed Beams;881
213.1;Abstract;881
213.2;1 Introduction;881
213.3;2 Focusing-Induced Polarization-State Changes;882
213.4;3 An Example: The Polarization Gating Pulse;882
213.5;4 Conclusions;883
213.6;Acknowledgement;883
213.7;References;883
214;200 Simultaneous Selective Two-Photon Microscopy Using MHz Rate Pulse Shaping and Quadrature Detection of the Time-Multiplexed Signal;885
214.1;Abstract;885
214.2;1 Introduction;885
214.3;2 Experimental;886
214.4;3 Results and Discussion;887
214.5;References;888
215;201 Simultaneous Spatial and Temporal Focusing of Femtosecond Laser Pulses for Directly Writing Optical Waveguides in Pr3+ Doped ZBLAN Glass;889
215.1;Abstract;889
215.2;1 Introduction;889
215.3;2 Experiments and Results;890
215.4;3 Conclusion;891
215.5;Acknowledgments;891
215.6;References;892mehr

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